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This collection is significant to researchers studying the history of Leon County, the history of the Florida State College for Women, and women's colleges because it documents the academic activities of Mary Simpson Yarbrough, who attended Florida State College for Women during the 1920s.

The Scarborough Papers include correspondence pertaining to mercantile business, land plats and deeds, a journal of mercantile business and plantation records. These materials about Scarborough's business afford a clear picture of early Florida merchandising and farming and contain many names of citizens of West Florida and of South Georgia. There are printed materials such as Hazeltine's almanac, The delineator and Literary digest. The 1907 Christmas issue of The delineator contains a number of Christmas songs, recipes and any amount of "styles of the month." The newspapers in the collection include six issues of The Sun, a Tallahassee, Florida, newspaper. These issues contain articles about the proposed project of draining the Everglades, and tobacco growing in Leon County.